I have had the problem you mention. Ctrl + C will work when R is able to realize "Oh, this guy/gal wants me to stop running that particular command." However, often R cannot do that. So you have to run Ctrl + \ (note that it's a backslash, not a forward slash). This tells Linux "Hey, R is not listening to me, can you stop running R?".
Try Ctrl + C first, because if it works you will still have your R session. If it doesn't work, and you do Ctrl + \ you will lose your R session, but at least it stops the process.
If that doesn't work either, then I would suggest a killall R
or a kill -9 [PID]
where you find the PID by running pus aux
.